We report the design, fabrication, and characterization of high-performance, solution-processed hybrid (inorganic-organic) light emitting transistors (HLETs). The devices employ a high-mobility, solution-processed cadmium sulfide layer as the switching and transport layer, with a conjugated polymer Super Yellow as an emissive material in non-planar source/drain transistor geometry. We demonstrate HLETs with electron mobilities of up to 19.5 cm2/V s, current on/off ratios of >107, and external quantum efficiency of 10−2% at 2100 cd/m2. These combined optical and electrical performance exceed those reported to date for HLETs. Furthermore, we provide full analysis of charge injection, charge transport, and recombination mechanism of the HLETs. The high brightness coupled with a high on/off ratio and low-cost solution processing makes this type of hybrid device attractive from a manufacturing perspective.
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3 November 2014
Research Article|
November 05 2014
High mobility solution-processed hybrid light emitting transistors
Bright Walker;
Bright Walker
a)
1School of Energy and Chemical Engineering,
Ulsan National Institute of Science and Technology
, Ulsan 689-798, South Korea
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Mujeeb Ullah;
Mujeeb Ullah
a)
2Centre for Organic Photonics & Electronics,
University of Queensland
, Brisbane, Queensland 4072, Australia
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Gil Jo Chae;
Gil Jo Chae
3Department of Materials Physics,
Dong-A University
, Busan 604-714, South Korea
4Department of Physics and EHSRC,
University of Ulsan
, Ulsan 680-749, South Korea
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Paul L. Burn;
Paul L. Burn
2Centre for Organic Photonics & Electronics,
University of Queensland
, Brisbane, Queensland 4072, Australia
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Shinuk Cho;
Shinuk Cho
4Department of Physics and EHSRC,
University of Ulsan
, Ulsan 680-749, South Korea
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Jin Young Kim;
Jin Young Kim
1School of Energy and Chemical Engineering,
Ulsan National Institute of Science and Technology
, Ulsan 689-798, South Korea
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Ebinazar B. Namdas;
Ebinazar B. Namdas
b)
2Centre for Organic Photonics & Electronics,
University of Queensland
, Brisbane, Queensland 4072, Australia
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Jung Hwa Seo
Jung Hwa Seo
b)
3Department of Materials Physics,
Dong-A University
, Busan 604-714, South Korea
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a)
B. Walker and M. Ullah contributed equally to this work.
b)
Authors to whom correspondence should be addressed. Electronic addresses: e.namdas@uq.edu.au and seojh@dau.ac.kr.
Appl. Phys. Lett. 105, 183302 (2014)
Article history
Received:
July 20 2014
Accepted:
October 21 2014
Citation
Bright Walker, Mujeeb Ullah, Gil Jo Chae, Paul L. Burn, Shinuk Cho, Jin Young Kim, Ebinazar B. Namdas, Jung Hwa Seo; High mobility solution-processed hybrid light emitting transistors. Appl. Phys. Lett. 3 November 2014; 105 (18): 183302. https://doi.org/10.1063/1.4900933
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