We report an effective method to remove the system-inherent background [Jungk et al., Appl. Phys. Lett. 91, 253511 (2007)] that is present in nominal piezoresponse force microscopy (PFM) setup. Control experiments performed in both ambient and ultrahigh vacuum environments indicate that the system-inherent background probably originates from the interactions between the modulation voltage and surface absorptions. By minimizing such interactions, background-free PFM results were obtained on glass, α-quartz, hexagonal ErMnO3, and periodically poled LiNbO3. The removal of background signal allows quantitative measurements of local intrinsic piezoelectric response with high sensitivity (0.1pm/V).

1.
J. F.
Scott
and
C. A. P.
Dearaujo
,
Science
246
,
1400
(
1989
).
2.
D.
Damjanovic
,
P.
Muralt
, and
N.
Setter
,
IEEE Sens. J.
1
,
191
(
2001
).
3.
N. G. R.
Broderick
,
G. W.
Ross
,
H. L.
Offerhaus
,
D. J.
Richardson
, and
D. C.
Hanna
,
Phys. Rev. Lett.
84
,
4345
(
2000
).
4.
N.
Amdursky
,
P.
Beker
,
J.
Schklovsky
,
E.
Gazit
, and
G.
Rosenman
,
Ferroelectrics
399
,
107
(
2010
).
5.
A.
Gruverman
and
S. V.
Kalinin
,
J. Mater. Sci.
41
,
107
(
2006
).
6.
S. V.
Kalinin
,
B. J.
Rodriguez
,
S.
Jesse
,
E.
Karapetian
,
B.
Mirman
,
E. A.
Eliseev
, and
A. N.
Morozovska
,
Annu. Rev. Mater. Res.
37
,
189
(
2007
).
7.
N.
Balke
,
I.
Bdikin
,
S. V.
Kalinin
, and
A. L.
Kholkin
,
J. Am. Ceram. Soc.
92
,
1629
(
2009
).
8.
J. A.
Christman
,
J. R. R.
Woolcott
,
A. I.
Kingon
, and
R. J.
Nemanich
,
Appl. Phys. Lett.
73
,
3851
(
1998
).
9.
M. H.
Zhao
,
Z. L.
Wang
, and
S. X.
Mao
,
Nano Lett.
4
,
587
(
2004
).
10.
T.
Jungk
,
A.
Hoffmann
, and
E.
Soergel
,
Appl. Phys. Lett.
91
,
253511
(
2007
).
11.
T.
Jungk
,
A.
Hoffmann
, and
E.
Soergel
,
Appl. Phys. Lett.
89
,
163507
(
2006
).
12.
Y.
Kumagai
,
A. A.
Belik
,
M.
Lilienblum
,
N.
Leo
,
M.
Fiebig
, and
N. A.
Spaldin
,
Phys. Rev. B
85
,
174422
(
2012
).
13.
P.
Guthner
and
K.
Dransfeld
,
Appl. Phys. Lett.
61
,
1137
(
1992
).
14.
T.
Hidaka
,
T.
Maruyama
,
M.
Saitoh
,
N.
Mikoshiba
,
M.
Shimizu
,
T.
Shiosaki
,
L. A.
Wills
,
R.
Hiskes
,
S. A.
Dicarolis
, and
J.
Amano
,
Appl. Phys. Lett.
68
,
2358
(
1996
).
15.
W.
Wang
,
J.
Zhao
,
W.
Wang
,
Z.
Gai
,
N.
Balke
,
M.
Chi
,
H. N.
Lee
,
W.
Tian
,
L.
Zhu
,
X.
Cheng
,
D. J.
Keavney
,
J.
Yi
,
T. Z.
Ward
,
P. C.
Snijders
,
H. M.
Christen
,
W.
Wu
,
J.
Shen
, and
X.
Xu
,
Phys. Rev. Lett.
110
,
237601
(
2013
).
16.
V. E.
Bottom
,
J. Appl. Phys.
41
,
3941
(
1970
).
17.
M.
Jazbinšek
and
M.
Zgonik
,
Appl. Phys. B: Lasers Opt.
74
,
407
(
2002
).
18.
S.
Lei
,
E. A.
Eliseev
,
A. N.
Morozovska
,
R. C.
Haislmaier
,
T. T. A.
Lummen
,
W.
Cao
,
S. V.
Kalinin
, and
V.
Gopalan
,
Phys. Rev. B
86
,
134115
(
2012
).
19.
T.
Choi
,
Y.
Horibe
,
H. T.
Yi
,
Y. J.
Choi
,
W.
Wu
, and
S.
Cheong
,
Nature Mater.
9
,
253
(
2010
).
20.
B. J.
Rodriguez
,
C.
Callahan
,
S. V.
Kalinin
, and
R.
Proksch
,
Nanotechnology
18
,
475504
(
2007
).
You do not currently have access to this content.