We aim to characterize the size distribution of nanoparticles located in the ablation plume produced by femtosecond laser interaction. The proposed method relies on the use of white-light extinction spectroscopy setup assisted by ultrafast intensified temporal gating. This method allows measurement of optical absorbance of a nickel nanoparticles cloud. Simulation of the extinction section of nickel nanoparticles size distributions has been developed in order to compare the measured optical absorbance to the optical extinction by theoretical and experimental nanoparticles size distributions (measured by scanning electron microscopy). A good agreement has been found between the in situ measured optical absorbance and the optical extinction cross section calculated from ex situ nanoparticles size distribution measurements.
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10 March 2014
Research Article|
March 10 2014
In situ diagnostic of the size distribution of nanoparticles generated by ultrashort pulsed laser ablation in vacuum
Florent Bourquard;
Florent Bourquard
Université de Lyon, CNRS UMR 5516, Laboratoire Hubert Curien, Université Jean Monnet
, Saint-Étienne, France
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Anne-Sophie Loir;
Anne-Sophie Loir
Université de Lyon, CNRS UMR 5516, Laboratoire Hubert Curien, Université Jean Monnet
, Saint-Étienne, France
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Christophe Donnet;
Christophe Donnet
Université de Lyon, CNRS UMR 5516, Laboratoire Hubert Curien, Université Jean Monnet
, Saint-Étienne, France
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Florence Garrelie
Florence Garrelie
a)
Université de Lyon, CNRS UMR 5516, Laboratoire Hubert Curien, Université Jean Monnet
, Saint-Étienne, France
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Florent Bourquard
Anne-Sophie Loir
Christophe Donnet
Florence Garrelie
a)
Université de Lyon, CNRS UMR 5516, Laboratoire Hubert Curien, Université Jean Monnet
, Saint-Étienne, France
a)
Author to whom correspondence should be addressed. Electronic mail: [email protected]
Appl. Phys. Lett. 104, 104101 (2014)
Article history
Received:
December 13 2013
Accepted:
February 26 2014
Citation
Florent Bourquard, Anne-Sophie Loir, Christophe Donnet, Florence Garrelie; In situ diagnostic of the size distribution of nanoparticles generated by ultrashort pulsed laser ablation in vacuum. Appl. Phys. Lett. 10 March 2014; 104 (10): 104101. https://doi.org/10.1063/1.4868103
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