Phytochemistry is one of the course in Chemistry Department’s curriculum which discusses about biosynthetic path of secondary metabolite compound in a plant, classification of secondary metabolite compound, isolation technique, and identification analysis. This course is expected to be able to bridge the generations of a nation that has expertise in managing the natural resources of Indonesian plants. In this research, it was evaluated the implementation of case study learning method towards students’ understanding on phytochemistry course. The learning processes were conducted in 2 cycles i.e. before and after midterm. The first seven themes of materials before midterm were learned with case study method and the next seven themes of materials were studied with the same method with the module-assisted. The results showed that there was enhancement of students’ understanding in class D that were obtained from comparison of midterm and final test. Contrarily, the students of class C have no significant enhancement. In addition, it was predicted that understanding enhancement was strongly influenced by the life skills and the motivation of students especially the academic skills aspect.

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