Several past research studies have demonstrated the fast fabrication of hygroscopic actuators using additive manufacturing (AM) technology. However, further insight is needed to assess the confounding effect of material types on the structure-property correlations in AM-produced hygroscopic bi-material actuators (BA). Premised on the above, this study sets out to quantify the responsiveness of BA produced by fused filament fabrication (FFF). The primary aim is to assess the influence of two FFF process parameters and the choice of materials on the BA’s responsiveness. In this vein, the investigation examined the effect of FFF’s layer height and extrusion width on the hygroscopic swelling coefficient of wood-filled polylactic acid polymers, pure polylactic acid (PLA) and thermoplastic polyurethane (TPU) polymers. Carried out also is the quantification of the hygromorphic response of monolithic FFF-printed BA derived from these materials. Deformation tests on the BA revealed its responsiveness to correlate positively with printing layer height, extrusion width, and the materials’ hygroscopic coefficient of expansion. Besides, the monolithic BA derived from the combination of the Wood-filled PLA/TPU composite specimens were found to generate mean/maximum tip deflections of 6.44 mm/9.5 mm, which are 4% and 11% more than what was obtained for the Wood-filled PLA/PLA composite specimens.

1.
Alshebly
,
Y.S.
,
M.
Nafea
,
M.S.M.
Ali
, and
H.A.
Almurib
,
Review on recent advances in 4D printing of shape memory polymers.
European Polymer Journal
,
2021
.
159
: p.
110708
.
2.
Mustapha
,
K.
and
K.M.
Metwalli
,
A review of fused deposition modelling for 3D printing of smart polymeric materials and composites.
European Polymer Journal
,
2021
.
156
: p.
110591
.
3.
Hsueh
,
C.
,
Thermal stresses in elastic multilayer systems.
Thin solid films
,
2002
.
418
(
2
): p.
182
188
.
4.
van Manen
,
T.
,
S.
Janbaz
, and
A.A.
Zadpoor
,
Programming 2D/3D shape-shifting with hobbyist 3D printers.
Mater Horiz
,
2017
.
4
(
6
): p.
1064
1069
.
5.
Hagaman
,
D.E.
,
S.
Leist
,
J.
Zhou
, and
H.F.
Ji
,
Photoactivated Polymeric Bilayer Actuators Fabricated via 3D Printing.
ACS Appl Mater Interfaces
,
2018
.
10
(
32
): p.
27308
27315
.
6.
Ruggeberg
,
M.
and
I.
Burgert
,
Bio-inspired wooden actuators for large scale applications.
PLoS One
,
2015
.
10
(
3
): p.
e0120718
.
7.
Dudescu
,
C.
and
L.
Racz
,
Effects of Raster Orientation, Infill Rate and Infill Pattern on the Mechanical Properties of 3D Printed Materials.
ACTA Universitatis Cibiniensis
,
2017
.
69
(
1
): p.
23
30
.
8.
Reyssat
,
E.
and
L.
Mahadevan
,
Hygromorphs: from pine cones to biomimetic bilayers.
J R Soc Interface
,
2009
.
6
(
39
): p.
951
7
.
9.
Reyssat
,
E.
and
L.
Mahadevan
,
Hygromorphs: from pine cones to biomimetic bilayers.
Journal of The Royal Society Interface
,
2009
.
6
(
39
): p.
951
957
.
10.
Correa
,
D.
,
S.
Poppinga
,
M.D.
Mylo
,
A.S.
Westermeier
,
B.
Bruchmann
,
A.
Menges
, and
T.
Speck
,
4D pine scale: biomimetic 4D printed autonomous scale and flap structures capable of multi-phase movement.
Philos Trans A Math Phys Eng Sci
,
2020
.
378
(
2167
): p.
20190445
.
11.
Li
,
P.
,
L.
Pan
,
D.
Liu
,
Y.
Tao
, and
S.Q.
Shi
,
A Bio-Hygromorph Fabricated with Fish Swim Bladder Hydrogel and Wood Flour-Filled Polylactic Acid Scaffold by 3D Printing.
Materials (Basel)
,
2019
.
12
(
18
).
12.
Le Duigou
,
A.
,
G.
Chabaud
,
F.
Scarpa
, and
M.
Castro
,
Bioinspired electro-thermo-hygro reversible shape-changing materials by 4D printing.
Advanced Functional Materials
,
2019
.
29
(
40
): p.
1903280
.
13.
Holstov
,
A.
,
B.
Bridgens
, and
G.
Farmer
,
Hygromorphic materials for sustainable responsive architecture.
Construction and Building Materials
,
2015
.
98
: p.
570
582
.
14.
Reichert
,
S.
,
A.
Menges
, and
D.
Correa
,
Meteorosensitive architecture: Biomimetic building skins based on materially embedded and hygroscopically enabled responsiveness.
Computer-Aided Design
,
2015
.
60
: p.
50
69
.
15.
Chen
,
X.
,
L.
Mahadevan
,
A.
Driks
, and
O.
Sahin
,
Bacillus spores as building blocks for stimuli-responsive materials and nanogenerators.
Nature Nanotechnology
,
2014
.
9
(
2
): p.
137
141
.
16.
Le Duigou
,
A.
and
M.
Castro
,
Hygromorph BioComposites: Effect of fibre content and interfacial strength on the actuation performances.
Industrial Crops and Products
,
2017
.
99
: p.
142
149
.
17.
Krapež Tomec
,
D.
,
A.
Straže
,
A.
Haider
, and
M.
Kariž
,
Hygromorphic Response Dynamics of 3D-Printed Wood-PLA Composite Bilayer Actuators.
Polymers
,
2021
.
13
(
19
).
18.
Le Duigou
,
A.
,
M.
Castro
,
R.
Bevan
, and
N.
Martin
,
3D printing of wood fibre biocomposites: From mechanical to actuation functionality.
Materials & Design
,
2016
.
96
: p.
106
114
.
19.
Kabir
,
S.M.F.
,
K.
Mathur
, and
A.-F.M.
Seyam
,
A critical review on 3D printed continuous fiber-reinforced composites: History, mechanism, materials and properties.
Composite Structures
,
2020
.
232
: p.
111476
.
20.
Balaraman
,
R.K.
,
S.
Hussain
,
J.K.
Ong
,
Q.Y.
Tan
,
U.-X.
Tan
, and
N.
Raghavan
,
Prediction of part density in additively manufactured maraging steel with supervised machine learning using pyrometer data.
Materials Today: Proceedings
,
2022
.
70
: p.
368
375
.
21.
Le Duigou
,
A.
,
D.
Correa
,
M.
Ueda
,
R.
Matsuzaki
, and
M.
Castro
,
A review of 3D and 4D printing of natural fibre biocomposites.
Materials & Design
,
2020
.
194
.
22.
Tezel
,
T.
,
V.
Kovan
, and
E.S.
Topal
,
Effects of the printing parameters on short-term creep behaviors of three-dimensional printed polymers.
Journal of Applied Polymer Science
,
2019
.
136
(
21
): p.
47564
.
23.
ISO
, Plastics-methods for determining the density of non-cellular plastics -- part 1: immersion method, liquid pyknometer method and titration method.
2004
,
International Organization for Standardization
:
Geneva
,
Switzerland
.
24.
Mustapha
,
K.B.
, Effects of Processing Parameters on the Characteristics of Additively Manufactured Polymeric Parts, in
Encyclopedia of Materials: Plastics and Polymers
,
M.S.J.
Hashmi
, Editor.
2022
,
Elsevier
:
Oxford
. p.
244
252
.
25.
Ayrilmis
,
N.
,
M.
Kariz
,
J.H.
Kwon
, and
M. Kitek
Kuzman
,
Effect of printing layer thickness on water absorption and mechanical properties of 3D-printed wood/PLA composite materials.
The International Journal of Advanced Manufacturing Technology
,
2019
.
102
(
5
): p.
2195
2200
.
This content is only available via PDF.
You do not currently have access to this content.