We theoretically study the enhancement of perovskite quantum dots nonlinear photoluminescence by resonant silicon nanoparticles. Using both numerical and analytical approaches, a multifold emission efficiency enhancement in CsPbBr3 perovskite nanocrystals is predicted. Namely, we reveal the enhancement of total Purcell Factor at emission wavelength by 10 times and averaged near-field enhancement at pump wavelength by 1.5 times. Our findings can be useful for up-conversion infrared light viewers and for bioimaging.
REFERENCES
1.
Nagamine
, G.
, Rocha
, J. O.
, Bonato
, L. G.
, Nogueira
, A. F.
, Zaharieva
, Z.
, Watt
, A. A.
, Carlos H. de Brito
Cruz
, & Padilha
, L. A.
(2018
). Two-photon absorption and two-photon-induced gain in perovskite quantum dots
. The Journal of Physical Chemistry Letters
, 9
(12
), 3478
–3484
.2.
Chen
, W.
, Bhaumik
, S.
, Veldhuis
, S. A.
, Xing
, G.
, Xu
, Q.
, Grätzel
, M.
, Mhaisalkar
, S.
, Mathews
, N.
, & Sum
, T. C.
(2017
). Giant five-photon absorption from multidimensional core-shell halide perovskite colloidal nanocrystals
. Nature Communications
, 8
(1
), 1
–9
.3.
Tiguntseva
, E. Y.
, Zograf
, G. P.
, Komissarenko
, F. E.
, Zuev
, D. A.
, Zakhidov
, A. A.
, Makarov
, S. V.
, & Kivshar
, Y. S.
(2018
). Light-emitting halide perovskite nanoantennas
. Nano Letters
, 18
(2
), 1185
–1190
.4.
Bayles
, A.
, Carretero-Palacios
, S.
, Calió
, L.
, Lozano
, G.
, Calvo
, M. E.
, & Míguez
, H.
(2020
). Localized surface plasmon effects on the photophysics of perovskite thin films embedding metal nanoparticles
. Journal of Materials Chemistry C.
5.
Makarov
, S.
, Furasova
, A.
, Tiguntseva
, E.
, Hemmetter
, A.
, Berestennikov
, A.
, Pushkarev
, A.
, Zakhidov
, A.
and Kivshar
, Y.
, 2019
. Halide-Perovskite Resonant Nanophotonics
. Advanced Optical Materials
, 7
(1
), p.1800784
.6.
Huang
, H.
, Bodnarchuk
, M. I.
, Kershaw
, S. V.
, Kovalenko
, M. V.
, & Rogach
, A. L.
(2017
). Lead halide perovskite nanocrystals in the research spotlight: Stability and defect tolerance
. ACS Energy Letters
, 2
(9
), 2071
–2083
.7.
Lu
, M.
, Zhang
, Y.
, Wang
, S.
, Guo
, J.
, Yu
, W. W.
, & Rogach
, A. L.
(2019
). Metal halide perovskite light-emitting devices: promising technology for next-generation displays
. Advanced Functional Materials
, 29
(30
), 1902008
.8.
Li
, B.
, Huang
, H.
, Zhang
, G.
, Yang
, C.
, Guo
, W.
, Chen
, R.
, Qin
, C.
, Gao
, Y.
, Biju
, V.P.
, Rogach
, A.L.
, Jia
, S.
, & Xiao
, L.
(2018
). Excitons and biexciton dynamics in single CsPbBr3 perovskite quantum dots
. The Journal of Physical Chemistry Letters
, 9
(24
), 6934
–6940
.9.
Zhang
, M.
, Wang
, M.
, Yang
, Z.
, Li
, J.
, & Qiu
, H.
(2018
). Preparation of all-inorganic perovskite quantum dots-polymer composite for white LEDs application
. Journal of Alloys and Compounds
, 748
, 537
–545
.10.
Tiguntseva
, E.
, Chebykin
, A.
, Ishteev
, A.
, Haroldson
, R.
, Balachandran
, B.
, Ushakova
, E.
, Komissarenko
, F.
, Wang
, H.
, Milichko
, V.
, Tsypkin
, A.
, Hu
, W.
, Makarov
, S.
, Zakhidov
, A.
, & Zuev
, D.
(2017
). Resonant silicon nanoparticles for enhancement of light absorption and photoluminescence from hybrid perovskite films and metasurfaces
. Nanoscale
, 9
(34
), 12486
–12493
.11.
Zhou
, B.
, Shi
, B.
, Jin
, D.
, & Liu
, X.
(2015
). Controlling upconversion nanocrystals for emerging applications
. Nature Nanotechnology
, 10
(11
), 924
.12.
Auzel
, F.
(2004
). Upconversion and anti-stokes processes with f and d ions in solids
. Chemical Reviews
, 104
(1
), 139
–174
.13.
Novotny
, L.
, & Hecht
, B.
(2012
). Principles of Nano-Optics
. Cambridge university press
.14.
Bohren
, C. F.
, & Huffman
, D. R.
(2008
). Absorption and scattering of light by small particles. John Wiley & Sons
.15.
Purcell
, E. M.
(1995
). Spontaneous emission probabilities at radio frequencies. In Confined Electrons and Photons
(pp. 839
–839
). Springer
, Boston, MA
.16.
Bharadwaj
, P.
, Deutsch
, B.
, & Novotny
, L.
(2009
). Optical antennas
. Advances in Optics and Photonics
, 1
(3
), 438
–483
.17.
Greffet
, J. J.
, Laroche
, M.
, & Marquier
, F.
(2010
). Impedance of a nanoantenna and a single quantum emitter
. Physical Review Letters
, 105
(11
), 117701
.18.
Chew
, H.
(1987
). Transition rates of atoms near spherical surfaces
. The Journal of Chemical Physics
, 87
(2
), 1355
–1360
.19.
Zyuzin
, M. V.
, Baranov
, D. G.
, Escudero
, A.
, Chakraborty
, I.
, Tsypkin
, A.
, Ushakova
, E. V.
, Florain
, K.
, Wolfgang
, J. P.
, & Makarov
, S. V.
(2018
). Photoluminescence quenching of dye molecules near a resonant silicon nanoparticle
. Scientific Reports
, 8
(1
), 1
–7
.20.
Ladutenko
, K.
, Pal
, U.
, Rivera
, A.
, & Peña-Rodríguez
, O.
(2017
). Mie calculation of electromagnetic near-field for a multilayered sphere
. Computer Physics Communications
, 214
, 225
–230
.21.
Greffet
, J. J.
, Laroche
, M.
, & Marquier
, F.
(2010
). Impedance of a nanoantenna and a single quantum emitter
. Physical Review Letters
, 105
(11
), 117701
.22.
Berestennikov
, A.S.
, Voroshilov
, P.M.
, Makarov
, S.V.
& Kivshar
, Y.S.
(2019
). Active meta-optics and nanophotonics with halide perovskites
. Applied Physics Reviews
, 6
(3
), 031307
.23.
Berestennikov
, A.S.
, Li
, Y.
, Iorsh
, I.V.
, Zakhidov
, A.A.
, Rogach
, A.L.
& Makarov
, S.V.
(2019
). Beyond quantum confinement: excitonic nonlocality in halide perovskite nanoparticles with Mie resonances
. Nanoscale
, 11
(14
), 6747
–6754
.24.
Tiguntseva
, E.
, Koshelev
, K.
, Furasova
, A.
, Tonkaev
, P.
, Mikhailovskii
, V.
, Ushakova
, E.V.
, Baranov
, D.G.
, Shegai
, T.
, Zakhidov
, A.A.
, Kivshar
, Y.
& Makarov
, S.V.
(2020
). Room-Temperature Lasing from Mie-Resonant Non-Plasmonic Nanoparticles
. ACS Nano
, DOI:
This content is only available via PDF.
© 2020 Author(s).
2020
Author(s)
You do not currently have access to this content.