In the paper in a class of regular harmonic functions we study properties of some integro-differential operators that generalize the operators of fractional differentiation in Hadamard sense. These operators transfer regular harmonic functions to the same function, and are inverse to the regular harmonic functions. Boundary value problem with the boundary operator of fractional order is studied in the exterior of the unit sphere. The considered problem generalizes the well-known Neumann problem on boundary operators of fractional order. We prove a theorem on existence and uniqueness of solutions of the problem. Moreover, an integral representation of the problem solution is obtained.

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